Surface chemistry of phase-pure M1 MoVTeNb oxide during operation in selective oxidation of propane to acrylic acid

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The impact of steam on the electronic structure of the selective propane oxidation catalyst MoVTeNb oxide (orthorhombic M1 phase).

The selective propane oxidation catalyst MoVTeNb oxide M1 was investigated by microwave conductivity, synchrotron X-ray photoelectron, soft X-ray absorption and resonant photoelectron spectroscopy under reaction conditions to identify the influence of steam on the electronic bulk and surface properties. Steam significantly increases both the conversion of propane and the selectivity to the targ...

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Selective oxidation of propane to acrylic acid with molecular oxygen

This review covers the recent developments and the present state of selective oxidation of propane to acrylic acid with molecular oxygen. The current commercial manufacturing process of acrylic acid, as well as the possible oxidation pathways of propane are included as background information. Special attention is given to three classes of leading catalysts: vanadium pyrophosphate, heteropoly ac...

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Effects of water on the catalytic performances of MoVTeNbO catalyst in the oxidation of propane to acrylic acid have been investigated at different reaction temperatures and different steam contents. Obtained results show that both catalytic performances and catalyst structure are very sensitive to the presence of water vapor in the reaction feed. Presence of water induces some structural modif...

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Effects of water on the catalytic performances of MoVTeNbO catalyst in the oxidation of propane to acrylic acid have been investigated at different reaction temperatures and different steam contents. Obtained results show that both catalytic performances and catalyst structure are very sensitive to the presence of water vapor in the reaction feed. Presence of water induces some structural modif...

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role of water in the partial oxidation of propane to acrylic acid over mo1v0.3te0.23nb0.12ox catalyst

effects of water on the catalytic performances of movtenbo catalyst in the oxidation of propane to acrylic acid have been investigated at different reaction temperatures and different steam contents. obtained results show that both catalytic performances and catalyst structure are very sensitive to the presence of water vapor in the reaction feed. presence of water induces some structural modif...

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ژورنال

عنوان ژورنال: Journal of Catalysis

سال: 2012

ISSN: 0021-9517

DOI: 10.1016/j.jcat.2011.09.012